The existence of the quantum spin liquid (QSL) state has fascinated physicists for decades. In 1973, physicist Phil Anderson hypothesized its presence in certain triangular lattices, but was unable to investigate further due to the lack of necessary tools. However, a recent breakthrough led by researchers from the Quantum Science Center (QSC) at the Oak Ridge National Laboratory has confirmed the existence of QSL behavior in a new material called KYbSe2. This discovery opens up new possibilities for the development of high-quality superconductors and quantum computing components.

Understanding Quantum Spin Liquid

QSLs are a unique state of matter controlled by the interactions among entangled magnetic atoms, known as spins. They excel at stabilizing quantum mechanical activity in materials like KYbSe2, which have layered triangular lattices. These materials are highly valued for their potential contributions to various technological advancements. Researchers have long been studying the triangular lattice structures of different materials in search of QSL behavior. KYbSe2 presents a unique advantage as its properties can be modified by swapping out atoms without changing its underlying structure.

The Research Process

The research team employed a combination of theoretical, experimental, and computational techniques to study QSL behavior in KYbSe2. By utilizing modern neutron scattering instruments, accurate measurements of complex materials at the atomic level were possible. The researchers observed multiple hallmarks of QSLs, such as quantum entanglement, exotic quasiparticles, and the proper balance of exchange interactions. The material was found to be close to the quantum critical point, which is favorable for QSL characteristics to thrive. The team also analyzed its single-ion magnetic state, using advanced spectrometers.

This groundbreaking study aligns with the QSC’s core priorities. Understanding QSLs is crucial for the development of next-generation technologies. The QSC aims to connect fundamental research to quantum electronics, quantum magnets, and other quantum devices. By identifying materials like KYbSe2 that have the potential to exhibit QSL behavior, researchers can modify and manipulate them to create small-scale devices from scratch. Although KYbSe2 is not a true QSL, a significant portion of its magnetism fluctuates at low temperatures, indicating the possibility of reaching a fully-fledged QSL state with slight alterations to its structure or external pressure.

The researchers’ findings have established an unprecedented protocol that can be applied to the study of other systems. They plan to conduct parallel studies and simulations on delafossite materials, further expanding our understanding of QSLs. By streamlining the evaluation process of QSL candidates, they hope to accelerate the search for genuine QSLs. This discovery in KYbSe2 marks a significant step towards harnessing the potential of QSLs for revolutionary technological advancements. As lead author Allen Scheie highlights, “we’ve found a way to orient ourselves on the map, so to speak, and show what we’ve gotten right.”

Physics

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